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The enantioselective addition of propargylic boronic acids to alpha-oxy-beta-ketoesters catalyzed by a new chiral Cu(II)-a-biscarboxylate ternary complex, and an optically pure tertiary amine, is described. With 1-(3,5-dimethylbenzyl)-2-propylamine or (+)-(R)-10-(2-phenylethyl)-2-(1-naphthyl)pyrrolidine as catalysts, (Z)-5-(1,3-dioxolan-2-yl)hexanoic acid ester is obtained in high yields with high enantioselectivities. Good functional group tolerance of the reaction is also demonstrated.Order Michigan Supreme Court
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I’m sorry that this has been more than a little disjointed, but I didn’t want to just write a post off of the cuff with no head start on my notes..
We’re asking for your help to make it through the offseason and. 1, Mike Trout*, 2011-2013, 1490.314.404.544, 166, 4024, 179. 2024.307.441.638, 511, 131, 157, 42, 151, 123, 110, 17, 176, -3, 7.4. We at FanGraphs promise to crack the whip so he can reduce that one-run-per-year error to zero.).
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